clock atomic nucleus crystal of calcium fluoride thorium
© Luca Toscani De Col/TU WienA crystal of calcium fluoride that is infused with thorium atoms (shown) is at the heart of a new nuclear clock.
Researchers already used one of the nuclear clocks to search for dark matter

For the first time, scientists used an atomic nucleus as a clock.

The world's most precise timepieces are made using atoms, specifically their electrons. But clocks based on atomic nuclei — protons and neutrons — might eventually outperform them, while also testing basic laws of physics in new ways. Now, the decades-old dream of a nuclear clock has finally been realized, two independent teams of researchers report.

The technology is still at an early stage, but the physics behind it is so different from that of atomic clocks that it's already broken new ground, researchers report in a paper submitted June 3 to arXiv.org. "In some types of measurements, we're already outperforming all of the atomic clocks," says physicist Thorsten Schumm of TU Wien in Vienna.

Schumm and colleagues used the clock to look for evidence of dark matter, the invisible, massive substance that is thought to pervade the universe. No signs of the shady stuff materialized, but the clock's estimated sensitivity to certain types of dark matter rivaled or beat that of atomic clocks.

"This is an outstanding result," says theoretical physicist Victor Flambaum of the University of New South Wales in Sydney, who was not involved with the research. And the feat should spur more progress: "This is only the first step. [The] race for building super-accurate nuclear clocks just started."

Nuclear clocks' potential to weigh in on dark matter and other exotic physics scenarios helps explains why, in this branch of physics, "nuclear clocks have become one of the most actively pursued frontiers," says Shiqian Ding of Tsinghua University in Beijing. In a study submitted June 7 to arXiv.org, Ding and colleagues describe their nuclear clock, which is based on similar technology to that of Schumm and colleagues. (Neither paper has been peer reviewed.)

At their hearts, both clocks consist of crystals of calcium fluoride imbued with thorium, which are probed with a laser. The two clocks showed similar performance. Ding and colleagues used a much more powerful laser, but Schumm and colleagues had more plentiful thorium in their crystal.

And thorium is key: In the entire periodic table, there's just a single type of atomic nucleus that can be used to make a clock: thorium-229. That's because the nucleus has to mesh well with the other major player, the laser.

In atomic and nuclear clocks, the wiggling electromagnetic waves of a laser's light act like the swinging pendulum in a grandfather clock. If that laser light weren't anchored to something steady, its frequency would drift over time, as if the grandfather clock's tick-tock slowed down or sped up. But in an atomic or nuclear clock, the laser's frequency is locked to a jump between energy levels for a particular atom or nucleus. For an atomic clock, the electrons make the jump, and for a nuclear clock, it's the nucleus. Thorium-229 is special because it's the only atomic nucleus with an energy jump that's the right size to be probed by a laser.

To lock a laser to an energy level jump, the laser must be frequently readjusted, using the outcome of measurements to determine how to nudge its frequency. In the new works, the two teams succeeded in implementing this feedback loop, a step that was absent in earlier demonstrations that laid the groundwork for a nuclear clock.

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